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An evaluation of models and computational approaches for the barrier properties of coatings containing flakes of high aspect ratio / A. Tsiantis in JOURNAL OF COATINGS TECHNOLOGY AND RESEARCH, Vol. 16, N° 2 (03/2019)
[article]
Titre : An evaluation of models and computational approaches for the barrier properties of coatings containing flakes of high aspect ratio Type de document : texte imprimé Auteurs : A. Tsiantis, Auteur ; T. D. Papathanasiou, Auteur Année de publication : 2019 Article en page(s) : p. 521-530 Note générale : Bibliogr. Langues : Américain (ame) Catégories : Matériaux -- Propriétés barrières
Paillettes
RevêtementsIndex. décimale : 667.9 Revêtements et enduits Résumé : We report on the results of a comprehensive two-dimensional computational study of diffusion across disordered flake composites. Our objective is (1) the evaluation of existing literature models for the effect of flake orientation and (2) the evaluation of the influence of boundary conditions and unit-cell types on the predicted barrier properties. Flake orientation is an important parameter affecting barrier properties in flake-filled composites, as the barrier efficacy of such systems depends significantly on the extent to which the flakes have been oriented as close as possible to being perpendicular to the direction of macroscopic diffusion. Our comparisons rely on an extensive set of computational results in two-dimensional, doubly periodic unit cells, each containing up to 3000 individual unidirectional flake cross-sections which are randomly placed and with their axes forming an angle (π/2 − θ) with the direction of macroscopic diffusion. A unique feature of our study is the consideration of high aspect ratio (α) systems with α = 100 and α = 1000, from the dilute (αφ = 0.01) and into the very concentrated (αφ = 40) regime. The effective diffusivity of the corresponding unit cells is computed from the imposed concentration difference and the computed mass flux, using Fick’s Law. We show that use of cyclic boundary conditions and doubly periodic unit cells results in effective diffusivities which are in agreement with theory and invariant of the shape of the unit cell. In addition, we show that the use of adiabatic boundary conditions produces erroneous results at high flake concentrations. Comparison of our results with existing theoretical models revealed several shortcomings of the latter concerning both the effect of flake concentration (αφ) and the effect of the orientation angle (θ). The principal reason for the latter shortcoming is the fact that said models do not respect the rotational invariance of the diffusivity tensor. Note de contenu : - COMPUTATIONAL
- RESULTS AND DISCUSSION : Effect of boundary conditions - Comparison to other relevant modelsDOI : 10.1007/s11998-018-0130-z En ligne : https://link.springer.com/content/pdf/10.1007%2Fs11998-018-0130-z Permalink : https://e-campus.itech.fr/pmb/opac_css/index.php?lvl=notice_display&id=32422
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Code-barres Cote Support Localisation Section Disponibilité 20894 - Périodique Bibliothèque principale Documentaires Disponible An investigation on usage of sodium borohydride and zinc oxide as oxygen scavengers in polyethylene terephthalate films / Ilhan Özen in INTERNATIONAL POLYMER PROCESSING, Vol. XXVII, N° 4 (08/2012)
[article]
Titre : An investigation on usage of sodium borohydride and zinc oxide as oxygen scavengers in polyethylene terephthalate films Type de document : texte imprimé Auteurs : Ilhan Özen, Auteur Année de publication : 2012 Article en page(s) : p. 493-497 Note générale : Bibliogr. Langues : Anglais (eng) Catégories : Borohydrure de sodium Le tétrahydruroborate de sodium, aussi appelé borohydrure de sodium, est un composé chimique constitué d'atomes de bore, de sodium et d'hydrogène. Sa formule brute est NaBH4.
C'est un agent réducteur utilisé notamment dans l'industrie pharmaceutique en tant que source d'hydrures H-. C'est un solide blanc, souvent rencontré sous forme de poudre.
Le borohydrure de sodium absorbe l'humidité de l'air (il est hygroscopique). Il réagit avec l'eau et dégage lentement du dihydrogène, un gaz inflammable/explosif. Selon la classification européenne des produits chimiques, il est enregistré avec la phrase de risque R14 "réagit violemment au contact de l'eau". Le produit se décompose à plus de 400 °C sans fondre. Sa décomposition est violente et exothermique avec l'eau.
Capteurs (technologie)
Films plastiques
Matériaux -- Propriétés barrières
Matières plastiques -- Extrusion:Polymères -- Extrusion
Oxyde de zinc
Oxygène
Polyéthylène téréphtalateIndex. décimale : 668.9 Polymères Résumé : The aim of this work is the production and characterisation of a plastic film having active oxygen barrier properties. The films have been obtained by adding an oxygen scavenger (either sodium borohydride (NaBH4) or zinc oxide (ZnO)) into a polyethylene terephthalate (PET) matrix during the extrusion process. In order to investigate the activity of the scavengers used, the produced films have been subjected to permeability measurements. It was revealed that NaBH4 – though a strong reductive agent – didn’t cause any degradation in matrix polymer but served as an ineffective oxygen scavenger as in the case of ZnO. DOI : 10.3139/217.2613 En ligne : https://drive.google.com/file/d/1MENbIXiAdGFiyS-MPffEdVC0bzu3w09T/view?usp=drive [...] Format de la ressource électronique : Permalink : https://e-campus.itech.fr/pmb/opac_css/index.php?lvl=notice_display&id=15773
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Code-barres Cote Support Localisation Section Disponibilité 14087 - Périodique Bibliothèque principale Documentaires Disponible Anticorrosion and barrier properties appraisal of poly(dimethylsiloxane)–ZnO nanocoating transition from superhydrophobic to hydrophobic state / Innocent O. Arukalam in JOURNAL OF COATINGS TECHNOLOGY AND RESEARCH, Vol. 16, N° 4 (07/2019)
[article]
Titre : Anticorrosion and barrier properties appraisal of poly(dimethylsiloxane)–ZnO nanocoating transition from superhydrophobic to hydrophobic state Type de document : texte imprimé Auteurs : Innocent O. Arukalam, Auteur ; Ying Li, Auteur Année de publication : 2019 Article en page(s) : p. 1077-1088 Note générale : Bibliogr. Langues : Américain (ame) Catégories : Anticorrosifs
Anticorrosion
Hydrophobie
Matériaux -- Propriétés barrières
Mouillabilité
Oxyde de zinc
Revêtements protecteurs
Test d'immersionIndex. décimale : 667.9 Revêtements et enduits Résumé : The anticorrosion and barrier properties of poly(dimethylsiloxane) (PDMS)–ZnO nanocoating transition from superhydrophobic to hydrophobic state have been evaluated. The main objective was to appraise the durability performance of anticorrosion and barrier properties of the pristine superhydrophobic coating and its hydrophobic state after long-term exposure to marine water. Thus, water wettability, surface features, and corrosion resistance, as well as barrier performance of the 1H, 1H, 2H, 2H-perfluorodecyltrichlorosilane-modified PDMS–ZnO coating were evaluated after 15 cycles (1 h to 60 days) of immersion in 3.5 wt.% NaCl solution. The evaluations were made by use of surface analytical, physicochemical, and electrochemical techniques. The results show that the coating transformed from superhydrophobic state (after 1 h) to hydrophobic state (after 60 days). The transition was due to effect of corrosiveness of the salty water and disappearance of the surface air layer with consequent reduction in the surface roughness and increase in the porosity of the coating. Correspondingly, the value of the impedance modulus decreased from 4.257 × 109 Ω cm2 (after 1 h) to 7.175 × 108 Ω cm2 (after 60 days). The trend of coating film (Rcf) and charge transfer (Rct) resistances with immersion time was found to be somewhat stable after 40-day immersion time. The observed high values of impedance modulus (|Z|f=0.01 Hz), Rcf and Rct after 60 days of immersion clearly demonstrate that the anticorrosion property and barrier performance of the transformed hydrophobic PDMS–ZnO coating were good. Note de contenu : - Wettability results of the coating
- Results of surface microstructure and roughness of the coating
- Chemical composition of the superhydrophobic PDMS-ZnO nanocoating
- Electrochemical impedance spectroscopy (EIS) results
- Effect of wetting and immersion time on the anticorrosion behavior of the coatingDOI : 10.1007/s11998-018-00182-2 En ligne : https://link.springer.com/content/pdf/10.1007%2Fs11998-018-00182-2.pdf Format de la ressource électronique : Permalink : https://e-campus.itech.fr/pmb/opac_css/index.php?lvl=notice_display&id=32863
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Code-barres Cote Support Localisation Section Disponibilité 21127 - Périodique Bibliothèque principale Documentaires Disponible Antimicrobial and improved barrier properties of natural phenolic compound-coated polymeric films for active packaging applications / Kirtiraj K. Gaikwad in JOURNAL OF COATINGS TECHNOLOGY AND RESEARCH, Vol. 16, N° 1 (01/2019)
[article]
Titre : Antimicrobial and improved barrier properties of natural phenolic compound-coated polymeric films for active packaging applications Type de document : texte imprimé Auteurs : Kirtiraj K. Gaikwad, Auteur ; Suman Singh, Auteur ; Youn Suk Lee, Auteur Année de publication : 2019 Article en page(s) : p. 147-157 Note générale : Bibliogr. Langues : Américain (ame) Catégories : Aliments -- Emballages
Antimicrobiens
Emballages en matières plastiques
Matériaux -- Propriétés barrières
Matériaux intelligents
Phénols
Polyéthylène basse densité
PyrogallolLe pyrogallol ou benzène-1,2,3-triol est un solide cristallin de couleur blanche utilisé comme réducteur en photographie.
En solution basique, il absorbe facilement l'eau, teintant une solution à l'origine incolore en violet. Le pyrogallol possède aussi des propriétés antiseptiques.
En chimie, du fait qu'il absorbe l'oxygène, il peut être utilisé pour piéger des traces d'oxygène résiduel dans un système devant rester anoxique, ou parfois encore pour mesurer le taux d'oxygène dans un mélange gazeux : par exemple dans l'appareil orsat.
Il a été et est encore parfois utilisé dans certaines teintures pour cheveux, mais cet usage est à présent restreint, le pyrogallol étant soupçonné d'être toxique.
Historiquement, le pyrogallol a servi de révélateur pour les tirages en noir et blanc. À quelques exceptions, pour des usages spécifiques, cet usage est grandement révolu et on préfère actuellement utiliser des développeurs comme l'hydroquinone.
RevêtementsIndex. décimale : 667.9 Revêtements et enduits Résumé : Functional antimicrobial low-density polyethylene (LDPE) films with coatings containing different amounts of pyrogallol (PGL), a natural phenolic substance, and polyurethane were prepared. To examine the applicability of the prepared LDPE/PGL films in packaging, the films were characterized by scanning electron microscopy, Fourier transform infrared, thermogravimetric analysis, and X-ray diffraction. The role of the coating, the barrier and color properties, and the antimicrobial activity of the films were evaluated. The thermal stability of the LDPE/PGL films was affected by the PGL concentration. Coatings with pyrogallol caused the barrier properties for water, and oxygen was increased from 0.78–0.32 to 470 ± 23.2–273 ± 57.1 (g mm)/(m2 h kPa), respectively. These findings indicate that the barrier properties of the LDPE/PGL films were highly improved compared to those of neat LDPE. Moreover, the LDPE/PGL films exhibited acceptable antimicrobial activity against Staphylococcus aureus (Gram-positive) and Escherichia coli (Gram-negative), especially for S. aureus. Further studies are necessary to increase the thermal stability of the pyrogallol coatings with the LDPE substrate in order to improve their performance and extend their packaging applications. Note de contenu : - MATERIALS AND METHODS : Materials - Film fabrication - Formation of pyrogallol coating
- CHARACTERIZATION : Scanning electron microscopy (SEM) - Fourier transform infrared (FTIR) - Thermogravimetric analysis - X-ray diffraction (XRD) - Water vapor permeability (WVP) - Oxygen transmission rate (OTR) - Color of films - UV–visible spectra - Antimicrobial activities of PGL-coated films
- RESULTS AND DISCUSSION : Scanning electron microscopy - Fourier transform infrared (FTIR) spectroscopy - Thermogravimetric analysis (TGA)- X-ray diffraction (XRD)- Water vapor permeability (WVP) - Oxygen transmission rate (OTR)- Color properties of films - UV–visible spectra - Antimicrobial activity
- Table 1 : Compositions of pyrogallol/polyurethane coatings with different amounts of pyrogallol
- Table 2 : Thermal stability of the LDPE/PGL films coated with different amounts of PGL
- Table 3 : WVP and OTR properties of the LDPE/PGL films
- Table 4 : Color values of the LDPE/PGL films coated with different amounts of PGLDOI : 10.1007/s11998-018-0109-9 En ligne : https://link.springer.com/article/10.1007/s11998-018-0109-9 Format de la ressource électronique : Permalink : https://e-campus.itech.fr/pmb/opac_css/index.php?lvl=notice_display&id=31978
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Code-barres Cote Support Localisation Section Disponibilité 20659 - Périodique Bibliothèque principale Documentaires Disponible Aqueous dispersions : high purity, easy-to-use coating additives / Alexandre Giardino Carmello in POLYMERS PAINT COLOUR JOURNAL - PPCJ, Vol. 204, N° 4594 (03/2014)
[article]
Titre : Aqueous dispersions : high purity, easy-to-use coating additives Type de document : texte imprimé Auteurs : Alexandre Giardino Carmello, Auteur ; Brian Prevo, Auteur Année de publication : 2014 Article en page(s) : p. 32-34-38 Note générale : Bibliogr. Langues : Anglais (eng) Catégories : Alumine
Latex
Matériaux -- Propriétés barrières
Oxydes métalliques
Polyacryliques
Poudres
Résistance à l'abrasion
Revêtements en phase aqueuse -- Additifs:Peinture en phase aqueuse -- Additifs
Rhéologie
SiliceLa silice est la forme naturelle du dioxyde de silicium (SiO2) qui entre dans la composition de nombreux minéraux.
La silice existe à l'état libre sous différentes formes cristallines ou amorphes et à l'état combiné dans les silicates, les groupes SiO2 étant alors liés à d'autres atomes (Al : Aluminium, Fe : Fer, Mg : Magnésium, Ca : Calcium, Na : Sodium, K : Potassium...).
Les silicates sont les constituants principaux du manteau et de l'écorce terrestre. La silice libre est également très abondante dans la nature, sous forme de quartz, de calcédoine et de terre de diatomée. La silice représente 60,6 % de la masse de la croûte terrestre continentale.Index. décimale : 667.9 Revêtements et enduits Résumé : The difficulty of handling, incorporating and dispersing some powder additives presents challenges to coating manufacturers employing such materials in their formulations. Furthermore, working with these powders can lead to some disadvantages including dirtiness and dust, contamination and possibly reduced performance.
Cab-O-Sperse fumed metal oxide dispersions can help balance or break some of the trade-offs between processing powder additives and the final performance of the coatings formulations in which those additives are used. Cab-0- Sperse dispersions use proprietary Cabot technology to produce highly stable fumed alumina or fumed silica dispersions in water, featuring uniform particle distributions with an average size of less than 0.2 pm, differing solid contents (12 to 40%), surface charges (anionic or cationic) and pH values (4 to 10.5). This results in several advantages compared to powder products, including ease of incorporation and mixing into liquid coatings, reduced dust in the environment, less waste and reduced risk of bubbling caused by trapped air. When used in coatings, the Cab-O-Sperse product line provides increased film hardness and abrasion resistance, improved corrosion resistance and barrier properties.
The Cab-O-Sperse dispersions line is presented below via comparative studies of formulations with no additives, formulations with rheological additives including dry fumed silica powder and formulations with added Cab-O-Sperse dispersions, in order to analyse their hardness, scratch resistance, transparency and rheological properties.Note de contenu : - An overview of fumed silica and fumed silica dispersions in coatings
- Polymer latex reinforcement by CAB-O-SPERSE dispersions
- Performance studies of waterborne acrylic coating containing CAB-O-SPERSE dispersionsEn ligne : https://drive.google.com/file/d/1_XDTYh0D0I8WBKm6IXAWx15os0WyOwJR/view?usp=drive [...] Format de la ressource électronique : Permalink : https://e-campus.itech.fr/pmb/opac_css/index.php?lvl=notice_display&id=20752
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